Search results for "Materials Science | Hot Paper"
showing 10 items of 1457 documents
Deep-Learning-Enabled Fast Optical Identification and Characterization of Two-Dimensional Materials
2019
Advanced microscopy and/or spectroscopy tools play indispensable role in nanoscience and nanotechnology research, as it provides rich information about the growth mechanism, chemical compositions, crystallography, and other important physical and chemical properties. However, the interpretation of imaging data heavily relies on the "intuition" of experienced researchers. As a result, many of the deep graphical features obtained through these tools are often unused because of difficulties in processing the data and finding the correlations. Such challenges can be well addressed by deep learning. In this work, we use the optical characterization of two-dimensional (2D) materials as a case stu…
Bulk sensitive photo emission spectroscopy of C1b compounds
2006
This work reports about bulk-sensitive, high energy photoelectron spectroscopy from the valence band of CoTiSb excited by photons from 1.2 to 5 keV energy. The high energy photoelectron spectra were taken at the KMC-1 high energy beamline of BESSY II employing the recently developed Phoibos 225 HV analyser. The measurements show a good agreement to calculations of the electronic structure using the LDA scheme. It is shown that the high energy spectra reveal the bulk electronic structure better compared to low energy XPS spectra.
Three addressable spin qubits in a molecular single-ion magnet
2016
We show that several qubits can be integrated in a single magnetic ion, using its internal electronic spin states with energies tuned by a suitably chosen molecular environment. This approach is illustrated with a nearly-isotropic Gd(III) ion entrapped in a polyoxometalate molecule. Experiments with microwave technologies, either three dimensional cavities or quantum superconducting circuits, show that this magnetic molecule possesses the number of spin states and the set of coherently addressable transitions connecting these states that are needed to perform a universal three-qubit processor or, equivalently, a d=8-level 'qudit'. Our findings open prospects for developing more sophisticate…
Nuclear quadrupole resonance spectroscopy with a femtotesla diamond magnetometer
2023
Sensitive Radio-Frequency (RF) magnetometers that can detect oscillating magnetic fields at the femtotesla level are needed for demanding applications such as Nuclear Quadrupole Resonance (NQR) spectroscopy. RF magnetometers based on Nitrogen-Vacancy (NV) centers in diamond have been predicted to offer femtotesla sensitivity, but published experiments have largely been limited to the picotesla level. Here, we demonstrate a femtotesla RF magnetometer based on an NV-doped diamond membrane inserted between two ferrite flux concentrators. The device operates in bias magnetic fields of 2-10 microtesla and provides a ~300-fold amplitude enhancement within the diamond for RF magnetic fields in the…
Inelastic neutron scattering due to acoustic vibrations confined in nanoparticles: theory and experiment
2008
The inelastic scattering of neutrons by nanoparticles due to acoustic vibrational modes (energy below 10 meV) confined in nanoparticles is calculated using the Zemach-Glauber formalism. Such vibrational modes are commonly observed by light scattering techniques (Brillouin or low-frequency Raman scattering). We also report high resolution inelastic neutron scattering measurements for anatase TiO2 nanoparticles in a loose powder. Factors enabling the observation of such vibrations are discussed. These include a narrow nanoparticle size distribution which minimizes inhomogeneous broadening of the spectrum and the presence of hydrogen atoms oscillating with the nanoparticle surfaces which enhan…
Tuning the effective spin-orbit coupling in molecular semiconductors
2017
The control of spins and spin to charge conversion in organics requires understanding the molecular spin-orbit coupling (SOC), and a means to tune its strength. However, quantifying SOC strengths indirectly through spin relaxation effects has proven diffi- cult due to competing relaxation mechanisms. Here we present a systematic study of the g-tensor shift in molecular semiconductors and link it directly to the SOC strength in a series of high mobility molecular semiconductors with strong potential for future devices. The results demonstrate a rich variability of the molecular g-shifts with the effective SOC, depending on subtle aspects of molecular composition and structure. We correlate t…
Speeding up of microstructure reconstruction: I. Application to labyrinth patterns
2011
Recently, entropic descriptors based the Monte Carlo hybrid reconstruction of the microstructure of a binary/greyscale pattern has been proposed (Piasecki 2011 Proc. R. Soc. A 467 806). We try to speed up this method applied in this instance to the reconstruction of a binary labyrinth target. Instead of a random configuration, we propose to start with a suitable synthetic pattern created by cellular automaton. The occurrence of the characteristic attributes of the target is the key factor for reducing the computational cost that can be measured by the total number of MC steps required. For the same set of basic parameters, we investigated the following simulation scenarios: the biased/rando…
Transversal spin freezing and re-entrant spin glass phases in chemically disordered Fe-containing perovskite multiferroics
2015
We propose experimental verification and theoretical explanation of magnetic anomalies in the complex Fe-contained double perovskite multiferroics like PbFe$_{1/2}$Nb$_{1/2}$O$_3$. The theoretical part is based on our model of coexistence of long-range magnetic order and spin glass in the above substances. In our model, the exchange interaction is anisotropic, coupling antiferromagnetically $z$ spin components of Fe$^{3+}$ ions. At the same time, the $xy$ components are coupled by much weaker exchange interaction of ferromagnetic sign. In the system with spatial disorder (half of corresponding lattice cites are occupied by spinless Nb$^{5+}$ ions) such frustrating interaction results in the…
Stable topological textures in a classical 2D Heisenberg model
2009
We show that stable localized topological soliton textures (skyrmions) with $\pi_2$ topological charge $\nu \geq 1$ exist in a classical 2D Heisenberg model of a ferromagnet with uniaxial anisotropy. For this model the soliton exist only if the number of bound magnons exceeds some threshold value $N_{\rm cr}$ depending on $\nu $ and the effective anisotropy constant $K_{\rm eff}$. We define soliton phase diagram as the dependence of threshold energies and bound magnons number on anisotropy constant. The phase boundary lines are monotonous for both $\nu=1$ and $\nu >2$, while the solitons with $\nu=2$ reveal peculiar nonmonotonous behavior, determining the transition regime from low to high …
Unraveling modular microswimmers: From self-assembly to ion-exchange-driven motors
2018
Active systems contain self-propelled particles and can spontaneously self-organize into patterns making them attractive candidates for the self-assembly of smart soft materials. One key limitation of our present understanding of these materials hinges on the complexity of the microscopic mechanisms driving its components forward. Here, by combining experiments, analytical theory, and simulations we explore such a mechanism for a class of active system, modular microswimmers, which self-assemble from colloids and ion-exchange resins on charged substrates. Our results unveil the self-assembly processes and the working mechanism of the ion-exchange driven motors underlying modular microswimme…